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020 ▼a 9780438304178
035 ▼a (MiAaPQ)AAI10827818
035 ▼a (MiAaPQ)uci:15196
040 ▼a MiAaPQ ▼c MiAaPQ ▼d 248032
0820 ▼a 540
1001 ▼a Karns, Alexander Sager.
24510 ▼a Investigation into the Dyotropic Rearrangement of Arene-Allene Cycloadducts, Studies Toward the Synthesis of Isonitrile-Containing Diterpene Natural Products, and Synthesis of Indolines via Cobalt(III)-Carbene Radical Catalysis.
260 ▼a [S.l.] : ▼b University of California, Irvine., ▼c 2018
260 1 ▼a Ann Arbor : ▼b ProQuest Dissertations & Theses, ▼c 2018
300 ▼a 437 p.
500 ▼a Source: Dissertation Abstracts International, Volume: 80-01(E), Section: B.
500 ▼a Adviser: Christopher D. Vanderwal.
5021 ▼a Thesis (Ph.D.)--University of California, Irvine, 2018.
520 ▼a Described herein is a compilation of studies in both methodology development and total synthesis in organic chemistry. Chapter 1 describes in detail notable discoveries in the field of dyotropic rearrangements, highlighting computational investi
520 ▼a Chapter 4 discusses in detail the isocyanoterpene natural products, including their proposed biogenesis, their observed bioactivity, and synthetic strategies by which they can be obtained in a laboratory setting. Chapter 5 elaborates specificall
520 ▼a Chapter 7 describes in detail the isolation of (+)-7,20-diisocyanoadociane and summarizes the total synthesis efforts toward the completed natural product. Chapter 8 highlights our improvements to our previously published formal synthesis of DIC
520 ▼a Chapter 9 provides a short summary of the field of cobalt(III)-carbene radical catalysis, including both mechanistic studies and applications to small molecule synthesis. Chapter 10 details our application of this unique reactivity to a rapid an
590 ▼a School code: 0030.
650 4 ▼a Chemistry.
690 ▼a 0485
71020 ▼a University of California, Irvine. ▼b Chemistry - Ph.D..
7730 ▼t Dissertation Abstracts International ▼g 80-01B(E).
773 ▼t Dissertation Abstract International
790 ▼a 0030
791 ▼a Ph.D.
792 ▼a 2018
793 ▼a English
85640 ▼u http://www.riss.kr/pdu/ddodLink.do?id=T14999078 ▼n KERIS
980 ▼a 201812 ▼f 2019
990 ▼a 관리자